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Introduction PART I: CONCEPTS AND TOOLS Non–Innocent Ligands Proton–Coupled Electron Transfer Reactions Computational Tools Multi–Site Catalysis / Catalysis by Multi–Nuclear Complexes Industrial Application of Molecular Base Metal Catalysis PART II: REACTIONS Carbenoid Insertion Reactions Nitrene Insertions Catalytic Water Oxidation Proton Reduction to Hydrogen Catalytic CO2 Reduction Catalytic Dehydrogenations Non–Reductive Reactions of CO2 Base Metal–Catalyzed C–C Cross–Couplings Base Metal–Catalyzed C–X Cross–Couplings (X=O, N, S) Hydrofunctionalization to Unsaturated Polar Bonds Hydrogenation of Polar Substrates Oxygenation of C=C and C–H Bonds Olefin Hydrogenation Reactions Reduction of N2 to NH3 Additions to Non–Polar C=C Bonds Directed C–H Bond Activation Catalytic Trifluoromethylation Using Base Metals Conjugate Additions Electrocyclic Reactions Oxidation of Polar Substrates